Magnetic ordering and spin reorientation in ErGa3
Chen, Y.Y. ; Yao, Y.D. ; Wang, C.R. ; Lin, S.H. ; Czopnik, A. ; Ali, M. R. ; Ho, J. C.
Chen, Y.Y.
Yao, Y.D.
Wang, C.R.
Lin, S.H.
Czopnik, A.
Ali, M. R.
Ho, J. C.
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2002-12-16
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Chen, Y., Yao, Y., Wang, C., Lin, S., Czopnik, A., Ali, M., & Ho, J. (2002). Magnetic ordering and spin reorientation in $\mathrmErGa_3$. Phys. Rev. B, 66, 212404.
Abstract
Calorimetric measurements between 0.3 and 10 K have been made on a single crystal of the AuCu3-type cubic compound ErGa3. The temperature dependence of specific heat exhibits an antiferromagnetic ordering-induced peak near 2.7 K, a second peak at 2.5 K due to spin reorientation, and a Schottky anomaly with crystal-field parameters x=0.17 and W=0.22 K, all in agreement with the results from neutron studies. The sum of the calculated entropies associated with the order-disorder process (R ln 2) and the crystal-field effect, respectively, is lower by 0.1R than the experimentally derived magnetic entropy values at approximately 6-10 K. This difference provides an estimate of a 2-J/mol latent heat for the spin rotation process. An anticipated transition from an amplitude-modulated magnetic structure to an equal magnetic-moment structure at temperatures near TN/2 was not observed.
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American Physical Society
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Physical Review B - Condensed Matter and Materials Physics
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0163-1829
